Effect of organic compounds on nanoparticle formation in diluted diesel exhaust

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Author(s) Mathis, Urs, Mohr, Martin E., Zenobi, Renato
Publication Type Journal Items, Publication Status: Published
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Title Effect of organic compounds on nanoparticle formation in diluted diesel exhaust
Author(s) Mathis, Urs
Mohr, Martin E.
Zenobi, Renato
Journal or Series Title Atmospheric chemistry and physics
Volume Number 4
Issue Number 3
Start Page 609
End Page 620
ISSN 1680-7316
1680-7324
Publisher European Geophysical Society
Publication Date 2004-04
Abstract The nucleation of nanoparticles in the exhaust of a modern light-duty diesel vehicle was investigated on a chassis dynamometer. This laboratory study is focused on the influence of volatile organic compounds (VOCs) on nucleation of volatile nanoparticles. Different organic compounds were added to the dilution air of the particle sampling under different sampling conditions. Sample temperature and relative sample humidity were varied in a wide range. The number size distribution of the particles was measured with a scanning mobility particle sizer (SMPS) and showed significant differences in response to the added organic compounds. While the nucleation mode particles showed a large variation in concentration, the accumulation mode particles remained unchanged for all compounds. Depending on the functional group, organic compounds were capable of initiating and increasing ( alcohols and toluene) or decreasing ( acetone, aniline, and methyl tert-butyl ether ( MTBE)) nucleation mode particles. Short volatile aliphatic hydrocarbons ( hexane and cyclohexane) turned out to be without effect on nucleation of nanoparticles. Possible reasons for the differences are discussed.
DOI 10.5194/acp-4-609-2004
Document Type Article
Publication Status Published
Language English
Assigned Organisational Unit(s) 03430
Organisational Unit(s)
NEBIS System Number 004294181
Source Database ID WOS-000220870900001
PP-9437
SCOPUS-3142520607
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@article{Mths2004,
  author = "Mathis, Urs and Mohr, Martin E. and Zenobi, Renato",
  title = "{E}ffect of organic compounds on nanoparticle formation in diluted diesel exhaust",
  journal = "Atmospheric chemistry and physics",
  year = 2004,
  volume = "4",
  number = "3",
  pages = "609--620",
  month = apr,
}


E-Citations record created: Fri, 13 Jul 2012, 12:08:42 CET