MALDI-Fourier transform mass spectrometric and theoretical studies of donor–acceptor and donor–bridge–acceptor fullerenes

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Author(s) Frankevich, Vladimir E., Dashtiev, Maxim, Zenobi, Renato, Kitagawa, Toshikazu, Lee, Yangsoo, Murata, Yasujiro, Yamazaki, Tetsuya, Gao, Yunyan, Komatsu, Koichi, Oliva, Josep M.
Publication Type Journal Items, Publication Status: Published
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Title MALDI-Fourier transform mass spectrometric and theoretical studies of donor–acceptor and donor–bridge–acceptor fullerenes
Author(s) Frankevich, Vladimir E.
Dashtiev, Maxim
Zenobi, Renato
Kitagawa, Toshikazu
Lee, Yangsoo
Murata, Yasujiro
Yamazaki, Tetsuya
Gao, Yunyan
Komatsu, Koichi
Oliva, Josep M.
Journal or Series Title Physical chemistry, chemical physics
Volume Number 7
Issue Number 5
Start Page 1036
End Page 1042
ISSN 1463-9076
1463-9084
Publisher The Royal Society of Chemistry
Publication Place Cambridge
Publication Date 2005
Abstract Fourier-transform ion cyclotron resonance (FTICR) mass spectrometric studies have been performed on donor - acceptor and donor - bridge - acceptor fullerene-based systems. Matrix-assisted laser desorption/ ionization (MALDI) was used for ion production; both the positive and negative ion modes were utilized. In addition, collision-induced dissociation (CID) experiments were carried out to study the movement of the charge ( electron or hole) upon fragmentation. The experiments are complemented by ab initio theoretical calculations yielding both molecular orbital energies and electron density distributions. It was found that the theoretical electron density map predicted the experimentally observed fragmentation correctly in every case. Both the calculations and the MS experiments may be useful in studying these and related donor-acceptor systems in view of their use for charge separation and eventually, solar energy production.
DOI 10.1039/b414349c
Additional Notes Received 16 September 2004, Accepted 12 January 2005, First published on the web 2 February 2005
Document Type Article
Publication Status Published
Language English
Assigned Organisational Unit(s) 03430
Organisational Unit(s)
NEBIS System Number 002005974
Source Database ID WOS-000227386700045
PP-17150
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@article{Frnkvch2005,
  author = "Frankevich, Vladimir E. and Dashtiev, Maxim and Zenobi, Renato and Kitagawa, Toshikazu and Lee, Yangsoo and Murata, Yasujiro and Yamazaki, Tetsuya and Gao, Yunyan and Komatsu, Koichi and Oliva, Josep M.",
  title = "{M}{A}{L}{D}{I}-{F}ourier transform mass spectrometric and theoretical studies of donor{\textendash}acceptor and donor{\textendash}bridge{\textendash}acceptor fullerenes",
  journal = "Physical chemistry, chemical physics",
  year = 2005,
  volume = "7",
  number = "5",
  pages = "1036--1042",
}


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